Ipzz-266 -

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exhibited a glass transition (T_g) at 112 °C, a modest increase relative to pristine P3HT (≈ 78 °C), consistent with the stiffening effect of ionic side‑chains.

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The convergence of ionic liquids (ILs) and conjugated polymers (CPs) has opened a promising route toward multifunctional materials that simultaneously transport ions and electrons. ILs possess negligible vapor pressure, high ionic conductivity, and wide electrochemical windows, whereas CPs such as polythiophene, polypyrrole, and poly(3,4‑ethylenedioxythiophene) (PEDOT) provide delocalized π‑electron pathways for electronic conduction. Merging these two families into a single polymeric scaffold—poly(ionic‑liquid) (PIL) composites—has demonstrated enhanced charge storage, mechanical robustness, and processability (see Ref. [1‑4]).

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